Black-carbon-induced regime transition of boundary layer development strongly amplifies severe haze

نویسندگان

چکیده

•High concentration of black carbon (BC) can trigger a tipping point PBL development•With aerosol load above the point, maximum height decreases abruptly•The is caused by BC-induced decoupling vertical mixing zones•Reducing BC much more efficient to avoid than reducing other aerosols Air pollution major threat human health. Severe haze often an unexpected extremely shallow planetary boundary layer (PBL), lowest part atmosphere where most pollutants are concentrated. Insufficient understanding formation mechanism leads failure air quality forecast and effective prevention. We found that high atmospheric concentrations black-carbon particles (an aerosol) “tipping point” in height. Above this these suppress layers create stable PBL, trapping near ground greatly deteriorating quality. This scenario be avoided through targeted reductions emissions (rather targeting total particulate matter reductions). Results further show mega-wildfires climate change nuclear disasters result enormous cause extreme stratification persistent layers. Black-carbon strongly influence (PBL) development thus severe formation, but its distinct role compared with scattering not yet fully understood. Here, combining numerical simulation field observation, we point,” daily abruptly when exceeding critical threshold optical depth (AOD), due zones. Because AOD increasing mass fraction, our results suggest abrupt transition adverse conditions below efficiently fraction increase (e.g., up four six times events Beijing). To achieve co-benefits for change, findings clearly demonstrate priority should given controlling emissions. In recent decades, heavy winter have frequently occurred Chinese megacity regions, threatening health millions.1Lelieveld J. Evans J.S. Fnais M. Giannadaki D. Pozzer A. The contribution outdoor sources premature mortality on global scale.Nature. 2015; 525: 367-371https://doi.org/10.1038/nature15371Crossref PubMed Scopus (3449) Google Scholar,2Zheng G.J. Duan F.K. Su H. Ma Y.L. Cheng Y. Zheng B. Zhang Q. Huang T. Kimoto Chang et al.Exploring Beijing: impact synoptic weather, regional transport heterogeneous reactions.Atmos. Chem. Phys. 15: 2969-2983https://doi.org/10.5194/acp-15-2969-2015Crossref (740) Scholar,3Cheng G. Wei C. Mu Wang Z. Gao He K. Carmichael al.Reactive nitrogen chemistry water as source sulfate during China.Sci. Adv. 2016; 2e1601530https://doi.org/10.1126/sciadv.1601530Crossref (789) Scholar,4Wang R. Gomez M.E. Yang L. Levy Zamora Hu Lin Peng Guo S. Meng al.Persistent from London Fog haze.Proc. Natl. Acad. Sci. USA. 113: 13630-13635https://doi.org/10.1073/pnas.1616540113Crossref (974) Scholar Light-absorbing aerosols, such (BC), radiation budget, leading cooling Earth’s surface near-surface warming overlying polluted atmosphere.5Ramanathan V. Crutzen P.J. Kiehl J.T. Rosenfeld Aerosols, climate, hydrological cycle.Science. 2001; 294: 2119-2124https://doi.org/10.1126/science.1064034Crossref (2958) Scholar,6Wilcox E.M. Thomas R.M. Praveen P.S. Pistone Bender F.A.-M. Ramanathan Black solar absorption suppresses turbulence layer.Proc. 11794-11799https://doi.org/10.1073/pnas.1525746113Crossref (88) Scholar,7Podgorny I.A. Conant W. Satheesh S.K. Aerosol modulation heating over tropical Indian Ocean.Tellus 2000; 52: 947-958https://doi.org/10.1034/j.1600-0889.2000.d01-4.xCrossref (126) Scholar,8Crutzen Birks J.W. after war: twilight at noon.Ambio. 1982; 11: 114-125Google also affects modulating snow albedo9Rahimi Liu X. Wu Lau W.K. Brown Qian Quantifying darkening radiative effects dust South Asian monsoon cycle: experiments using variable-resolution CESM.Atmos. 2019; 19: 12025-12049https://doi.org/10.5194/acp-19-12025-2019Crossref (26) Scholar,10Wei Lu Zhao Rahimi Xia Jiang carbon-climate interactions regulate burdens India revealed COVID-19.Nat. Commun. 2022; 13: 1839https://doi.org/10.1038/s41467-022-29468-1Crossref (8) large-scale circulations.11Lau K.M. Kim M.K. summer anomalies induced direct forcing: Tibetan Plateau.Clim. Dyn. 2006; 26: 855-864https://doi.org/10.1007/s00382-006-0114-zCrossref (830) Scholar,12Yang Smith S.J. Lou Rasch Impact anthropogenic emission injection uncertainty sulfur dioxide distribution.J. Geophys. Res. Atmos. 124: 4812-4826https://doi.org/10.1029/2018JD030001Crossref (10) Although has been widely recognized important agent budget forcing,13Jacobson M.Z. Strong state aerosols.Nature. 409: 695-697https://doi.org/10.1038/35055518Crossref (1942) Scholar,14Andreae M.O. dark side 671-672https://doi.org/10.1038/35055640Crossref (137) Scholar,15Bond T.C. Doherty Fahey D.W. Forster P.M. Berntsen DeAngelo B.J. Flanner M.G. Ghan Kärcher Koch al.Bounding system: scientific assessment.J. 2013; 118: 5380-5552https://doi.org/10.1002/jgrd.50171Crossref (3943) Scholar,16Ackerman T.P. A model effect urban climates particular applications Los Angeles Basin.J. 1977; 34: 531-547https://doi.org/10.1175/1520-0469Crossref still troposphere directly influenced surface. common definition which presence lower detectable.17Lenschow D.H. Probing Atmospheric Boundary Layer. Amer Meteorological Society, 1986Crossref During daytime, convective largely driven convections closely linked turbulent diffusion pollutants. Several studies will alter strength, thermal stability, development, aggravate pollution.5Ramanathan Scholar,18Wendisch Hellmuth O. Ansmann Heintzenberg Engelmann Althausen Eichler Müller al.Radiative dynamic absorbing Pearl River Delta, China.Atmos. Environ. 2008; 42: 6405-6416https://doi.org/10.1016/j.atmosenv.2008.02.033Crossref (55) Scholar,19Ding A.J. Nie Sun J.N. Kerminen V.-M. Petäjä Y.F. X.-Q. M.H. al.Enhanced megacities China.Geophys. Lett. 43: 2873-2879https://doi.org/10.1002/2016GL067745Crossref (519) Scholar,20Huang Ding aerosol-PBL interaction pollution: multiyear observational evidences North 2018; 45: 8596-8603https://doi.org/10.1029/2018GL079239Crossref (154) Scholar,21Dickerson R.R. Kondragunta Stenchikov Civerolo K.L. Doddridge B.G. Holben B.N. ultraviolet photochemical smog.Science. 1997; 278: 827-830https://doi.org/10.1126/science.278.5339.827Crossref (479) Scholar,22Xing Mathur Pleim Hogrefe Gan C.-M. Wong D.C. Hao Unexpected benefits effects.Environ. Technol. 50: 7527-7534https://doi.org/10.1021/acs.est.6b00767Crossref Scholar,23Wong Binkowski F. Otte Gilliam Pouliot Xiu Young J.O. Kang WRF-CMAQ two-way coupled system feedback: software preliminary results.Geosci. Model Dev. (GMD). 2012; 5: 299-312https://doi.org/10.5194/gmd-5-299-2012Crossref (163) Scholar,24Liu Fedorovich E. X.-M. Lee shortwave entrainment layer: large-eddy study.J. 9: 347-799https://doi.org/10.3390/atmos9090347Crossref Scholar,25Liu statistics spectra study.Atmosphere. 347https://doi.org/10.3390/atmos9090347Crossref On hand, lift top compensating reduced buoyancy underneath.26Yu Dickinson R.E. Radiative evolution layer.J. Res-Atmos. 2002; 107: AAC 3-1-AAC 3-14https://doi.org/10.1029/2001JD000754Crossref Scholar,27Rudich Sagi Influence Kuwait oil fires plume (1991) microphysical clouds.J. 2003; 1084478https://doi.org/10.1029/2003jd003472Crossref (35) Scholar,28Barbaro Vilà-Guerau de Arellano Krol M.C. Holtslag A.A.M. Impacts dynamics idealized layer.Bound-Lay. Meteorol. 148: 31-49https://doi.org/10.1007/s10546-013-9800-7Crossref (46) Scholar,29Li Liao Xue Zhu boundary-layer quality.Natl. Rev. 2017; 4: 810-833https://doi.org/10.1093/nsr/nwx117Crossref (453) Scholar,30Jacobson Studying photolysis rate coefficient temperature profiles airshed.J. 1998; 103: 10593-10604https://doi.org/10.1029/98jd00287Crossref (176) Moreover, light within may lead rather strengthened stratification.31Tie R.-J. Cao Pöschl U. Hoffmann Dusek al.Severe China amplified moisture.Sci. Rep. 715760https://doi.org/10.1038/s41598-017-15909-1Crossref (152) cloud distribution via aerosol-cloud aerosol-radiation interactions,32Twomey albedo 1149-1152https://doi.org/10.1175/1520-0469(1977)034<1149:tiopot>2.0.co;2Crossref Scholar,33Ding Tan Zhou al.Aerosol-boundary-layer-monsoon amplify semi-direct biomass smoke low Southeast Asia.Nat. 2021; 12: 6416https://doi.org/10.1038/s41467-021-26728-4Crossref (23) energy balance well meteorology cloud. revisit topic comprehensive investigations single-column simulations Weather Research Forecasting (WRF) online WRF (WRF-Chem), wide range scenarios different meteorological properties (concentration, single-scattering [SSA], distribution) studied (Figure S1). find sharp regime explains amplifies regions northern China. Figure 1A shows response structure (AOD) under stagnant weather SSA = 0.85, characteristic Beijing Plain (see (Hmax) (black line 1A) loads exceed certain (AOD ∼ 1.2), suggesting regimes. According long-term statistics,34Xie Dong Lv Bai Daily estimation ground-level PM2.5 beijing 3 km resolution MODIS AOD.Environ. 49: 12280-12288https://doi.org/10.1021/acs.est.5b01413Crossref (249) Scholar,35Zheng Shi Chen Qiu Analysis influential factors relationship between Beijing.Atmos. 17: 13473-13489https://doi.org/10.5194/acp-17-13473-2017Crossref (136) ∼1.2 area corresponds, average, fine (PM2.5) ∼100–200 μg m−3 winter.34Xie (blue dashed marks two regimes interaction. low-AOD ≤ almost no Hmax. When crossing threshold, 0.1 unit drop Hmax ∼600 ∼200 m, showing strong PBL. Such evident similar prompt heat exchange coefficients (Kh, colored contour 1A), reflect intensity mixing, key parameter dispersion best knowledge, first time collapse revealed. As shown Figures 1B, unique feature light-absorbing aerosols. Increasing non-absorbing (i.e., 1.0, purely scattering) only continuous moderate reduction Kh (Figures 1B S2). importance AOD. 1C, decreasing fraction) 0.8 0.95 factor ∼2, probability aerosol-induced decrease Further sensitivity both WRF-Chem models that, existence limited specific conditions, distributions, or scheme locations, seasons S3A–S3C, S3H, S3I, S4, S5), commonly existing mechanism. value different, always observed. results, weaker higher tendency S3B, S3D, S3E), means play wintertime 2A observed daytime loading Beijing, based micropulse lidar (MPL) measurements December, January, February December 2016 2018 section “experimental procedures”). For comparison, performed column same period procedures” supplemental information). accordance 2B 2C), observations exhibit (∼0.5–0.75) period, modeled around 50% exceeds consistent observation 2A). These support proposed development). contrast conventional interactions, gradual expected net (Rn) sensible flux (Fh), S8, Rn Fh do against BC. Then, question why does respond differently AOD? answer understand underlying mechanism, investigated diurnal below, around, S9). indicated Kh, zones: one heating, another altitude At SSA, it zone dimming effect29Li gradient atmosphere. promotes upper providing additional inducing convection S10A). invigoration layered aviation biomass-burning plumes.36Radke L.F. Lyons J.H. Hobbs P.V. Weiss Smokes burning fuel their self-lofting heating.J. 1990; 95: 14071-14076https://doi.org/10.1029/JD095iD09p14071Crossref Scholar,37Boers Laat A.T. Stein Zweers Dirksen R.J. Lifting potential solar-heated layers.Geophys. 2010; 37https://doi.org/10.1029/2010GL045171Crossref Scholar,38de A.T.J. Boers Tuinder O.N.E. escalator: evidence self-lifting 2009 Australian Saturday plume.J. 117https://doi.org/10.1029/2011jd017016Crossref Scholar,39Lelieveld Klingmüller Burnett R.T. Haines Effects fossil removal public climate.Proc. 116: 7192-7197https://doi.org/10.1073/pnas.1819989116Crossref (336) 3A 3B), zones each course reaching m noontime. despite upper-level (actually heating; S10A) S8A), uniform θ 15:00 clear proof able eliminate dilute emitted upward blue lines 2E). long coupled, increased inter-zonal compensates zone, insensitive mean 1A, S2, S3F, S3G). (SSA 1.0), terms “suppressing” regime, and, increases 0.8), even slightly enhance prior S2 S4). 3C 3D), suppressed so cannot connect one. interactions. Under condition, large difference, forms noontime inversion afternoon (orange red 3E S11). After decoupling, 1.5, ∼530 while shallower ∼190 m. stronger suppression BC-containing explained reasons: (1) first, incoming radiation, heating. absorbed lost reach anymore, scattered reflected back space rest S8A, extinction (the sum absorption), less (2) reduces flux. heats bottom air, resulting driving difference So, smaller S8B), zone. decoupled > trapped start ∼100-m requires 0.5-unit elevated fractions 0.85), ∼1.7-unit 1.0). attributed three factors: forward ratio, S5); atmosphere, air-surface fluxes S9B); residual morning, retarding full Our finding reconciles contrasting early studies, 3A) corresponds weak slight PBL,5Ramanathan whereas effect6Wilcox Scholar,40Liu Xie Yu Tian P. Lowe summertime.Environ. 14124003https://doi.org/10.1088/1748-9326/ab4872Crossref (17) Scholar,41Liu Bi al.Efficient layer.Geophys. 2020; 47e2020GL088858https://doi.org/10.1029/2020GL088858Crossref (20) 4B). upper-air necessarily stratification, regime. However, once decoupled, suppressed, form. unfavorable condition resembles nighttime 1A). help explain nonlinear dependence levels; By reanalyzing data al.,19Ding

برای دانلود باید عضویت طلایی داشته باشید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Simulation of boundary layer transition induced by periodically passing wakes

By X I A O H U A W U , R O B E R T G. J A C O B S , J U L I A N C. R. H U N T 2 AND P A U L A. D U R B I N 1 Center for Integrated Turbulence Simulations, Flow Physics and Computation Division, Department of Mechanical Engineering, Stanford University, Building 500, Stanford, CA 94305-3030, USA e-mail: [email protected]; [email protected]; [email protected] Department of App...

متن کامل

Temporal variations of black carbon during haze and non-haze days in Beijing

Black carbon (BC) aerosol has been identified as one of key factors responsible for air quality in Beijing. BC emissions abatement could help slow regional climate change while providing benefits for public health. In order to quantify its variations and contribution to air pollution, we systematically studied real-time measurements of equivalent black carbon (eBC) in PM2.5 aerosols at an urban...

متن کامل

Roughness Induced Transition in a Supersonic Boundary Layer

Direct numerical simulation is used to investigate the transition induced by threedimensional isolated roughness elements in a supersonic boundary layer at a free stream Mach number of 3.5. Simulations are performed for two different configurations: one is a square planform roughness and the other is a diamond planform roughness. The mean-flow calculations show that the roughness induces counte...

متن کامل

Compressible boundary layer transition induced by isolated roughness elements

The laminar-to-turbulent transition of boundary layers induced by isolated threedimensional roughness elements is analyzed by mining a direct numerical simulation database, which covers the variation of many physical parameters, including Mach and Reynolds numbers, and obstacle shape and size. We find that the transition process is approximately controlled by a Reynolds number based on the mome...

متن کامل

Compressibility Effects on Roughness-induced Boundary Layer Transition

Direct numerical simulation is used to investigate the effect of compressibility on roughness-induced boundary layer transition. Computations are performed in both the lowand the high-speed regime (at free-stream Mach number Me = 2) for an isolated three-dimensional element with cubic shape and for two-dimensional roughness strips. For each configuration two values of the roughness height Reyno...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

ژورنال

عنوان ژورنال: One earth

سال: 2023

ISSN: ['2590-3322', '2590-3330']

DOI: https://doi.org/10.1016/j.oneear.2023.05.010